Advancements in 2D material manipulation have led to new material science possibilities, notably with self-intercalation of metal atoms into transition metal dichalcogenides.
Manipulation of intercalation ratios significantly impacts atomic structure and physical properties of materials like iron selenide (Fe1+xSe2).
Researchers at Peking University demonstrated how slight intercalation ratio changes affect atomic ordering and properties in Fe1+xSe2.
Self-intercalation inserts additional Fe atoms into TMDs' van der Waals gaps, creating new materials with enhanced properties.
A systematic approach to intercalation revealed relationships between intercalation ratios, atomic structures, and magnetic behaviors.
Experiments showed varying Fe1+xSe2 compositions resulting in disordered, half-ordered, and fully ordered structures based on intercalated forms.
Innovative methods like space confinement-assisted chemical potential regulation provided precise control over intercalation levels.
Magnetic property changes were observed in synthesized materials based on intercalation states, affecting magnetoresistance behaviors.
Atomic structure manipulation through intercalation led to the creation of new materials with tunable structural and magnetic traits.
This research paves the way for designing next-generation materials with tailored properties, promising applications in electronics and spintronics.